Papers by Keyword: Random Laser

Abstract: Diatoms are unicellular aquatic microalgae possessing amazing self-assembled ordered micro-and nanoporous hierarchical silica cell walls called frustules. The quasi-periodic and highly regular pore patterns on the diatom surface are very attractive for applications based on optical and photonic properties of materials. The present contribution reports on pioneering research aimed at explore the multiple scattering and localization of light shown by diatom frustules in order to amplify their photoluminescence in a random laser (RL), as this technology is highly attractive for medical diagnostics and other advanced applications. RL is a special type of laser in which the optical feedback is due to light scattering in an amplifying medium instead of a conventional optical cavity. We have studied a set of selected frustules with different shapes and pore patterns, obtained from diatom cultivation in large scale photobioreactors, for comparative analysis of their random lasing effect in the bioscaffold soaked with organic dyes having luminescence in the visible range. Taking advantage from a multidisciplinary approach combining expertise from biology, physics and materials sciences, relying on high-resolution instrumentation and advanced algal cultivation equipment the results about random laser emission in the composite material were obtained. This will allow going ahead in the research aimed to the application to photonic devices in the field of medicine and medical diagnostic.

Abstract: The observation of random laser (RL) with coherent feedback in transparent polymer films based on Rh6G-PVP by spin-coating was carried out in the present investigation. Some sharp peaks with FWHM identified to be 2 nm appeared on the fluorescent spectra of polymer films which pumped by Nd:YLF pulse laser (wavelength: 526nm, frequence: 1Hz, pulse duration: 1ns, energy power: 1.2mJ/pulse). The threshold of emission spectra is ~35 and the spectra range from 570 ~ 610 nm. Streak camera was used to record the temporal process of RLs and the pulse duration time was measured to ~400ps. Rh6G-PVP transparent films were a kind of polymer films with numerous nanogaps distributed randomly on the surface of the film. The photons will be multiple scatterred and amplified during the spreading in the polymer film owing to the refractive index difference between nanogaps and polymer films. As the Rh6G-PVP polymer films have characters of convenient fabrication processes, low threshold and low cost, it shows great potential application in photoelectron and laser imaging.

Abstract: The random lasing emission from granular-surface PS:PMMA:Alq3:DCJTB blend films was investigated. By micro-phase separation of PS:PMMA:Alq3:DCJTB blend in spin-coating and solvent evaporation process, we obtained a granular-surface waveguide film with gain on glass substrates, whose period is about 200~500nm, and fluctuation is about 20nm. Pumped by THG YAG laser, a significant random laser emission was observed. Compared with the samples of glass/PMMA:Alq3:DCJTB and glass/ PS:Alq3:DCJTB prepared under the same conditions, the laser threshold decreased about 5 times, the line width at half (FWHM) reduced to 1.7nm from more than ten nm, and the quality factor of laser peak increased 7-9 times.

Abstract: We investigated the lasing spectra of multiple scattering active media based on solid polymer solutions of rhodamin 6G with embedded scattering silica particles of mean diameter 500nm. Lasing in these samples appears without any cavity and arises even in rather small active volume 0.05*0.5*0.5mm3. In a thick sample positive feedback for lasing is provided mainly by multiple scattering of light. In a thin sample the feedback is provided both by multiple scattering of light on the particles and light reflection from the sample surface. It is found that the lasing spectra peak wavelength can be varied within 13nm by varying sample thickness in a range 0.1 -1.65mm. A method of continuos laser tuning by wedge-like sample shift with respect to the pump beam is proposed. The presented results are aimed at the development of a new type of microlaser.