Authors: Hidefumi Shimoyama, Tokiko Osawa, Hiromi Watanabe, Kosuke Suzuki, Hiroshi Sakurai, Masahisa Ito
Abstract: Co/Pd magnetic multilayers have been prepared by using a sputtering method. Lattice distances and magnetic hysteresis curves have been measured by X-ray diffraction (XRD) measurements and magnetization measurements using a vibrating sample magnetometer (VSM). The XRD measurements have shown that the samples with thinner Pd layers have shorter lattice distances, and the VSM measurements have shown that the samples of thinner Co and thicker Pd layers are closer to those of perpendicular magnetic anisotropy. We have applied the X-ray magnetic diffraction method to the Co/Pd multilayer for the first time and have succeeded in observing a change in the X-ray diffraction intensities by the reversal of the magnetization direction.
3
Authors: Masahisa Ito, Kosuke Suzuki, Hiroshi Sakurai, Ryutaro Yamaki, Ayako Sato, Masayoshi Itou, Yoshiharu Sakurai
Abstract: We have applied two kinds of experimental methods using elliptically polarized synchrotron X-rays, magnetic Compton and Bragg scattering experiments, to a single crystal of a disordered Pd0.80Co0.20 alloy, and have measured magnetic Compton profiles and magnetic form factors, respectively. The result of the Compton scattering experiment has shown that the electronic structure of Pd0.80Co0.20 is similar to that of Pd0.72Co0.28, and the spin moment has been evaluated. The result of the Bragg scattering experiment has reinforced that of the previous experiment [M. Ito et al.: Mater. Sci. Forum Vol. 459 (2011), p. 3.], and the spin moment estimated by the magnetic Bragg scattering has reproduced that by the magnetic Compton scattering. These results show that the joint study of the magnetic Compton and Bragg scattering provides a tool for investigating the magnetic property of alloys.
39
Authors: Masahiro Naito, Kenta Hiiragi, Ayako Sato, Hiroshi Maruyama, Masahisa Ito
Abstract: We have performed X-ray magnetic diffraction experiments of a ferromagnetic binary alloy Fe3Pt in order phase, and have measured separately spin and orbital magnetic form factors. By a curve-fitting analysis in which atomic-model form factors of Fe-3d and Pt-5d electrons under the dipole approximation are assumed, we have obtained the spin and orbital magnetic moments of Fe and Pt atoms separately. The present result is comparable to those of other experimental and theoretical studies, which shows the validity of this experimental method.
3
Authors: Masahisa Ito, Ryota Nagayasu, Tatsuki Tadenuma, Kosuke Suzuki, Ayako Sato, Hiromichi Adachi, Yoshiharu Sakurai, Yoshichika Ōnuki
Abstract: An experimental method of X-ray magnetic diffraction was applied to the ferromagnetic rare-earth compound CeRh3B2, and its spin and orbital magnetic form factors were measured independently for the first time. Our curve-fitting analysis shows that the orbital magnetic form factor is reproduced by the calculated atomic-model form factor of Ce-4f electrons under the dipole approximation. The comparison of the sum of form factors and the total magnetic form factor measured by the polarized neutron diffraction reveals anisotropic distribution of the magnetic moment in real space.
3
Authors: Kosuke Suzuki, Masahisa Ito, Naruki Tsuji, Hiromichi Adachi, Hironori Nakao, Youichi Murakami, Yasujiro Taguchi, Yoshinori Tokura, Eiji Nishibori, Makoto Sakata
Abstract: An X-ray magnetic diffraction (XMD) is applied to ferromagnetic transition metal oxide YTiO3. The spin magnetic form factors are measured for 81 reciprocal lattice points of h0l, hk0 and 0kl series. Three-dimensional spin density distribution in the real space of YTiO3 is successfully obtained by using Maximum Entropy Method (MEM). This is the first result of spin density in the real space by the XMD.
7
Authors: Masahisa Ito, Yoshiaki Oba, Ayako Sato, Kosuke Suzuki, Tatsuki Tadenuma, Ryota Nagayasu, Hiroshi Sakurai, Hiromichi Adachi
Abstract: We have measured spin and orbital magnetic form factors of Pd3Co for various reciprocal lattice points by the X-ray magnetic diffraction. Observed spin and orbital magnetic form factors are fitted by theoretical curves of the isolated atomic model under the dipole approximation. By the fitting analysis we have evaluated separately the spin and orbital component of the magnetic moment of Pd3Co alloy as 2.19 µB/f.u. and 0.83 µB/f.u., respectively. The total magnetic moment 3.02 µB/f.u. is comparable to the value of 2.93 µB/f.u. obtained by the magnetization measurement.
3