The in situ deposition of SiNx masks by metal-organic vapour phase epitaxy was
optimized to achieve c-plane oriented GaN layers on sapphire having a dislocation
density of less than 2 x 108/cm2. The defect termination was found to be most
efficient if the SiNx was located after the growth of 100nm GaN, whereas when
deposited directly onto the AlN nucleation it was less efficient but yielded highly
compressively strained layers indicated by a donor-bound exciton peak position of
3.493eV in photoluminescence (13K). Furthermore it was observed via in situ reflectometry that a higher deposition temperature during the silane treatment
strongly increased the surface roughening to yield faster coalescence during the
GaN overgrowth but finally influenced the defect termination negatively. In terms
of lateral overgrowth, a high V/III ratio (2D growth mode) was most efficient in
terms of defect reduction, whereas a 3D–2D-process at lower V/III ratio yielded
much faster overgrowth but influenced the defect termination negatively.
Process Optimization for the Effective Reduction of Threading Dislocations in
MOVPE Grown GaN Using in situ Deposited SiNx Masks. J.Hertkorn, F.Lipski,
P.Brückner, T.Wunderer, S.B.Thapa, F.Scholz, A.Chuvilin, U.Kaiser, M.Beer,
J.Zweck: Journal of Crystal Growth, 2008, 310[23], 4867-70