Transmission electron microscope observations were used to analyze
microstructures in a (11•0)-plane GaN thin films grown by metal-organic vapourphase
epitaxy (MOVPE) onto a r (1¯1•2)-plane sapphire substrate Special attention
was paid to an influence of small off-angle of the substrate plane to morphology of
defects in the thin films. From the TEM observations, the following conclusions
were drawn. (1) The crystallographic orientation relationship between GaN and
sapphire substrate was (11•0)[00•1][¯11•0]GaN||(1¯1•2)[¯11•1][11•0]sapphire. The
direction of +c -polarity coincides with that reported previously. (2) The pits on the
surface were formed on the grain boundaries of GaN. (3) The density of pits was
related with the density of nucleation of GaN-islands on the substrate. The increase
in density of pits with the off-angle can be explained by the increase of nucleation
sites provided by atomic steps on the substrate. (4) The side-wall planes of pits and
voids were considered to be closed to ±(00•1), ±(11•4), and (11•2). (5) The
formation of pits and voids were attributable to the trend that such inclining planes
as (11•2) and (11•4) were stable compared with +c (00•1). A possible technique for
reduction of defects was also discussed.
Off-Angle Dependence of Void Formation and Defect Behavior in a-Plane
MOVPE-GaN on r-Plane Sapphire Substrate. N.Kuwano, A.Fukushima,
Y.Kugiyama, T.Ezaki, M.Minami, M.Araki, K.Hoshino, K.Tadatomo: Physica
Status Solidi C, 2009, 6[S2], S494-7