The BaCe0.8Pr0.2O3-α ceramic was synthesized by high temperature solid-state
reaction. The structural characteristics and the phase purity of the crystal were
determined using powder X-ray diffraction analysis. By using the methods of AC
impedance spectroscopy, gas concentration cell and electrochemical pumping of
hydrogen, the conductivity and ionic transport number of BaCe0.8Pr0.2O3-α were
measured, and the electrical conduction behavior of the material was investigated
in different gases at 500 to 900C. The results indicate that the material was of a
single perovskite-type orthorhombic phase. From 500 to 900 C, electronic-hole
conduction was dominant in dry and wet oxygen, air or nitrogen, and the total
conductivity of the material increased slightly with increasing oxygen partial
pressure in the oxygen partial pressure range studied. Ionic conduction was
dominant in wet hydrogen, and the total conductivity was about one or two orders
of magnitude higher than that in hydrogen-free atmosphere (oxygen, air or
nitrogen).
Mixed Conduction in BaCe0.8Pr0.2O3-α Ceramic. M.Y.Wang, L.G.Qiu: Chinese
Journal of Chemical Physics, 2008, 21[3], 286-90