The oxygen vacancy in BiFeO3 was calculated to be a double donor with states
0.6eV below the conduction band edge, consistent with cathodoluminescence and
electronic conductivity data. The atomic configurations were relaxed using the
local density approximation plus Hubbard U (LDA+U) to the electron-correlation
energy for each defect charge state to ensure that the oxide had a non-zero bandgap.
The defect formation energies were calculated using the screened exchange
functional.
Energy Levels of Oxygen Vacancies in BiFeO3 by Screened Exchange. S.J.Clark,
J.Robertson: Applied Physics Letters, 2009, 94[2], 022902