A simple chemical precipitation technique was used to synthesize europium-doped
cerium oxide nanostructures so as to enhance the emission properties. Structural
and optical studies revealed an sharp dependence upon the concentration of oxygen
ion vacancies and trivalent cerium which, in turn, could be modified by the dopant
concentration and the annealing temperature. The results of X-ray photo-electron
spectroscopy revealed an increase, in the tetravalent cerium concentration, to 85%
upon annealing at 900C. The concentration of oxygen ion vacancies increased from
1.7 x 1020 to 4.1 x 1020/cm3 with an increase in dopant concentration. The
maximum emission at room temperature was obtained for 15mol%Eu-doped ceria,
and improved with annealing temperature.
Luminescence Properties of Europium-Doped Cerium Oxide Nanoparticles: Role
of Vacancy and Oxidation States. A.Kumar, S.Babu, A.S.Karakoti, A.Schulte,
S.Seal: Langmuir, 2009, 25[18], 10998-1007