Spatially resolved X-ray fluorescence maps were presented that showed the
introduction and the evolution of oxygen vacancies in chromium-doped strontium
titanate during an electric-field-driven insulator-to-metal transition. The vacancies
were introduced at the anode and diffuse through the crystal toward the cathode.
The spatial distribution of vacancies was explained by a model describing the
electrical breakdown as a percolation process. Strong differences in the vacancy
distribution were found when the transition took place in air and in a hydrogenenriched
atmosphere. In air, the vacancies disappeared from the surface, whereas in
the reducing hydrogen atmosphere, they remained at the surface.
Spatial Distribution of Oxygen Vacancies in Cr-Doped SrTiO3 During an Electric-
Field-Driven Insulator-to-Metal Transition. B.P.Andreasson, M.Janousch,
U.Staub, G.I.Meijer: Applied Physics Letters, 2009, 94[1], 013513