TiO2-B nanowires were synthesized by an ion exchanging-thermal treatment. The
unique morphology of pits and dislocations interspersed on TiO2-B nanowires were
firstly characterized and studied by high-resolution transmission electron
microscopy. Oriented attachment was suggested as an important growth
mechanism in the evolvement of pits and dislocations on TiO2-B nanowires.
Lattice shears and fractures were originally formed during the ion exchanging
process of the sodium titanate nanowires, which resulted in the formation of
primary crystalline units and vacancies in the layered hydrogen titanate nanowires.
Then the (110) lattice planes of TiO2-B grown in [110] direction was faster than the
other lattice planes, which caused the exhibition of long dislocations on TiO2-B
nanowires. The enlargement of the vacancies, which was caused by the
rearrangement of primary crystalline units, should be the reason of the formation of
pits. Additionally, the transformation from TiO2-B to anatase could be also
elucidated by oriented attachment mechanism.
The Evolvement of Pits and Dislocations on TiO2-B Nanowires Via Oriented
Attachment Growth. B.Zhao, F.Chen, W.Qu, J.Zhang: Journal of Solid State
Chemistry, 2009, 182[8], 2225-30