Argon diffusivities and solubilities in single, gem-quality crystals of forsterite,
enstatite and quartz were deduced from experiments conducted under 0.5 to
~6000bar Ar pressures at 425 to 1200C. Surface-sensitive analyses were used to
confirm that the near-surface regions of the crystals were crystalline, unreacted and
free from structural damage. Polished single-crystal slabs and specimens with
natural facets were placed in open containers and exposed to an argon atmosphere
either in a pressure vessel or in a gas-flow tube furnace at near-atmospheric
pressure. Argon atoms from the pressure medium diffused into the crystals to
produce near-surface concentration gradients, which were directly profiled using
Rutherford back-scattering spectrometry. The following Arrhenius relationships
were obtained:
forsterite: D (m2/s) = 7.2 x 10-20exp[-42(kJ/mol)/RT]
enstatite: D (m2/s) = 1.3 x 10-20exp[-32(kJ/mol)/RT]
quartz: D (m2/s) = 3.1 x 10-19exp[-43(kJ/mol)/RT]
These activation energies were suspected to be apparent ones that were a
combination of the effects of the lattice diffusion of Ar atoms and trapping in
point-defect vacancies. There were no discernible differences in Ar diffusion in
different crystallographic directions, and the diffusivities did not vary as a function
of the intrinsic oxygen fugacity of the experimental vessels. The uptake gradients
also yielded Ar lattice solubilities, as represented by the concentrations at the
mineral surfaces. There were small differences between the solubilities in forsterite
and quartz, but all of the solubilities were high: ~2000ppm[wt]. The Ar solubilities
for iron-bearing enstatite and San Carlos olivine were much higher than for the
other minerals. The mean value for enstatite was 30 to 60% higher than for ironfree
minerals. This was attributed to the incorporation of Ar in point defects that
were more abundant in enstatite due to the oxidation of minor FeO contents. The
Ar solubilities were independent of pressure above ~1bar, but were slightly lower
at 0.5 to 1bar. This suggested that all of the sites capable of accommodating Ar
atoms were filled at pressures of ~1bar. In all cases, Ar appeared to be compatible;
although the degree of compatibility was expected to depend upon the minimum Ar
fugacity required to fully populate the available vacancies.
Lattice Diffusion and Solubility of Argon in Forsterite, Enstatite, Quartz and
Corundum. J.B.Thomas, D.J.Cherniak, E.B.Watson: Chemical Geology, 2008,
253[1-2], 1-22