AgI nanowires/anodic aluminium oxide (AgI NWs/AAO) composites were
fabricated by a simple approach, which involves the thermal melting of AgI
powders on the surface of the AAO membrane, followed by the infiltration of the
molten AgI inside the nanochannels. As-prepared AgI nanowires have corrugated
outer surfaces and were polycrystalline according to scanning electron microscopy and transmission electron microscopy observations. X-ray diffraction showed that a
considerable amount of 7H polytype AgI exists in the composites, which was
supposed to arise from the interfacial interactions between the embedded AgI and
the alumina. AC conductivity measurements for the AgI nanowires/AAO
composites exhibit a notable conductivity enhancement by three orders of
magnitude at room temperature compared with that of pristine bulk AgI.
Furthermore, a large conductivity hysteresis and abnormal conductivity transitions
were observed in the temperature-dependent conductivity measurements, from
which an ionic conductivity as high as 8.0 x 102S/cm was obtained at around 70C
upon cooling. The differential scanning calorimetry result demonstrated a similar
phase transition behaviour as that found in the AC conductivity measurements. The
enhanced ionic conductivity, as well as the abnormal phase transitions, can be
explained in terms of the existence of the highly conducting 7H polytype AgI and
the formation of well-defined conduction paths in the composites.
Enhanced Ionic Conductivity of AgI Nanowires/AAO Composites Fabricated by a
Simple Approach. L.F.Liu, S.W.Lee, J.B.Li, M.Alexe, G.H.Rao, W.Y.Zhou,
J.J.Lee, W.Lee, U.Gösele: Nanotechnology, 2008, 19[49], 495706