A permeation cell was used to measure rates of H permeation through arc-cast material of better than 3N-purity. The permeation was measured at temperatures ranging from 1300 to 2600C, and at H pressure differentials of 1 and 0.1atm; across isothermal W membranes (table 195). The H permeation rates were almost proportional to the square root of the pressure, were inversely proportional to the membrane thickness, and obeyed:
P (cm mm/min atm½) = 33.2 exp[-33.0(kcal/mol)/RT]
E.A.Aitken, H.C.Brassfield, P.K.Conn, E.C.Duderstadt: Transactions of the Metallurgical Society of AIME, 1967, 239[10], 1565-74
Table 195
Permeation of H through Arc-Cast W
T (C) | Pressure Gradient (atm) | P (cm mm/min atm½) |
1300 | 1 | 0.0013 |
1500 | 1 | 0.0023-0.0033 |
1500 | 0.1 | 0.00094-0.0031 |
1540 | 1 | 0.0032 |
1540 | 0.1 | 0.0038 |
1800 | 1 | 0.010-0.012 |
1840 | 1 | 0.011 |
1840 | 0.1 | 0.010 |
2000 | 1 | 0.021-0.025 |
2000 | 0.1 | 0.021-0.022 |
2040 | 1 | 0.024 |
2200 | 1 | 0.033-0.043 |
2200 | 0.1 | 0.041 |
2240 | 1 | 0.042 |
2240 | 0.1 | 0.042 |
2400 | 1 | 0.054-0.071 |
2400 | 0.1 | 0.052-0.071 |
2440 | 1 | 0.070 |
2500 | 1 | 0.064-0.088 |
2500 | 0.1 | 0.063-0.086 |
2600 | 1 | 0.078-0.11 |
2600 | 0.1 | 0.071-0.11 |