Effects of Chlorine on Disinfection by-Products (DBPs) Formation in Synthetic Drinking Water

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This study focused on the effect of chlorine on disinfection by-product (DBPs) formation. The concentration of DBPs and total residual chlorine were measured at the same time in synthetic drinking water. Chlorine demand and DBPs increased with chlorine dose and contact time. The descending DBPs formation potential rank was: TCM > DCAA > TCAA > TCNM > BDCM. Furthermore, a linear relation between the concentrations of DBPs (HAAs, THMs or TNMs) and chlorine demand was discovered, and the coefficients did not correlate with chlorine dose. Emerging N-DBPs such as HANs did not follow those disciplines because of their special structures. These results have instructive meanings to the further control of DBPs.

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492-496

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February 2013

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© 2013 Trans Tech Publications Ltd. All Rights Reserved

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[1] Bond, T., et al., Occurrence and control of nitrogenous disinfection by-products in drinking water - A review. WATER RESEARCH, 2011. 45(15): pp.4341-4354.

DOI: 10.1016/j.watres.2011.05.034

Google Scholar

[2] Plewa, M.J., et al., Occurrence, synthesis, and mammalian cell cytotoxicity and genotoxicity of haloacetamides: An emerging class of nitrogenous drinking water disinfection byproducts. ENVIRONMENTAL SCIENCE & TECHNOLOGY, 2008. 42(3): pp.955-961.

DOI: 10.1021/es071754h

Google Scholar

[3] Plewa, M.J., et al., Occurrence, synthesis, and mammalian cell cytotoxicity and genotoxicity of haloacetamides: An emerging class of nitrogenous drinking water disinfection byproducts. ENVIRONMENTAL SCIENCE & TECHNOLOGY, 2008. 42(3): pp.955-961.

DOI: 10.1021/es071754h

Google Scholar

[4] Muellner, M.G., et al., Haloacetonitriles vs. regulated haloacetic acids: Are nitrogen-containing DBPs more toxic? ENVIRONMENTAL SCIENCE & TECHNOLOGY, 2007. 41(2): pp.645-651.

DOI: 10.1021/es0617441.s001

Google Scholar

[5] Xie, Y.F., D.A. Reckhow and D.C. Springborg, Analyzing HAAs and ketoacids without diazomethane. JOURNAL AMERICAN WATER WORKS ASSOCIATION, 1998. 90(4): pp.131-138.

DOI: 10.1002/j.1551-8833.1998.tb08416.x

Google Scholar

[6] Liu, W. and S. Qi, Modeling and verifying chlorine decay and chloroacetic acid formation in drinking water chlorination. FRONTIERS OF ENVIRONMENTAL SCIENCE & ENGINEERING IN CHINA, 2010. 4(1): pp.65-72.

DOI: 10.1007/s11783-010-0010-y

Google Scholar

[7] Peretyazhko, T. and G. Sposito, Reducing capacity of terrestrial humic acids. GEODERMA, 2006. 137(1-2): pp.140-146.

DOI: 10.1016/j.geoderma.2006.08.004

Google Scholar

[8] Brown, D., J. Bridgeman and J.R. West, Predicting chlorine decay and THM formation in water supply systems. REVIEWS IN ENVIRONMENTAL SCIENCE AND BIO-TECHNOLOGY, 2011. 10(1): pp.79-99.

DOI: 10.1007/s11157-011-9229-8

Google Scholar

[9] Fooladvand, M., et al., Investigation of trihalomethanes formation potential in Karoon River water, Iran. ENVIRONMENTAL MONITORING AND ASSESSMENT, 2011. 178(1-4): pp.63-71.

DOI: 10.1007/s10661-010-1672-4

Google Scholar

[10] Shah, A.D. and W.A. Mitch, Halonitroalkanes, Halonitriles, Haloamides, and N-Nitrosamines: A Critical Review of Nitrogenous Disinfection Byproduct Formation Pathways. ENVIRONMENTAL SCIENCE & TECHNOLOGY, 2012. 46(1): pp.119-131.

DOI: 10.1021/es203312s

Google Scholar

[11] Krasner, S.W., et al., Occurrence of a new generation of disinfection byproducts. ENVIRONMENTAL SCIENCE & TECHNOLOGY, 2006. 40(23): pp.7175-7185.

Google Scholar

[12] Richardson, S.D., Disinfection by-products and other emerging contaminants in drinking water. TRAC-TRENDS IN ANALYTICAL CHEMISTRY, 2003. 22(10): pp.666-684.

DOI: 10.1016/s0165-9936(03)01003-3

Google Scholar