Characterization of Semi-Refined Carrageenan Reinforced with Cellulose Nanofiber Incorporated α-Tocopherol for Active Food Packaging Applications

Article Preview

Abstract:

This work focuses on the development of biodegradable active films packaging using natural compounds by reducing the plastic waste to environment but also as a potential substitute of synthetic preservative in food. Active film packaging was formulated using semi-refined carrageenan (SRC) biopolymer plasticized with glycerol (G), reinforced with different concentrations cellulose nanofiber (CNF) at 0 to 13% w/w incorporated 0.4% w/w α-tocopherol as natural antioxidants. Physical and mechanical properties of the film samples were analyzed. Active films reinforced CNF enhanced overall the tensile strength and the value of elongation at break significantly (p<0.05). Film samples reinforced with 10% w/w CNF improved the value of opacity, thickness, films solubility (%) and moisture content (%) with (5.60±0.14, 0.139 ±0.02, 27.89±2.41 and 18.88±1.06) respectively. In summary, an active film with 10% w/w CNF showed highest improvement on the mechanical and physical properties due to the uniform dispersion between CNF-SRC matrix interactions. Hence, the new formulation of active packaging film with showed competitive properties that could be an alternative solution for biodegradable films with function of food protection against oxidative degeneration.

You might also be interested in these eBooks

Info:

Periodical:

Materials Science Forum (Volume 1007)

Pages:

154-159

Citation:

Online since:

August 2020

Export:

Price:

Permissions CCC:

Permissions PLS:

Сopyright:

© 2020 Trans Tech Publications Ltd. All Rights Reserved

Share:

Citation:

* - Corresponding Author

[1] N. Benbettaïeb, T. Karbowiak, S. Bornaz, F. Debeaufort, Spectroscopic analyses of the influence of electron beam irradiation doses on mechanical, transport properties and microstructure of chitosan-fish gelatin blend films, Food Hydrocolloids, 46 (2015) 37-51.

DOI: 10.1016/j.foodhyd.2014.09.038

Google Scholar

[2] D. K. Takma, F. Korel, Active packaging films as a carrier of black cumin essential oil: Development and effect on quality and shelf-life of chicken breast meat, Food Packaging and Shelf Life, 19 (2019) 210-217.

DOI: 10.1016/j.fpsl.2018.11.002

Google Scholar

[3] K. H. A. Hamid, W. A. W. Yahaya, N. A. Z. M Saupy, M. P. Almajano, N. A. M. Azman, Semi‐refined carrageenan film incorporated with α‐tocopherol: Application in food model, J. Food Process. Preserv. 43(5) (2019) e13937.

DOI: 10.1111/jfpp.13937

Google Scholar

[4] A. Farhan, N. M. Hani, Characterization of edible packaging films based on semi-refined kappa-carrageenan plasticized with glycerol and sorbitol, Food Hydrocolloids, 64 (2017) 48-58.

DOI: 10.1016/j.foodhyd.2016.10.034

Google Scholar

[5] E. Sogut, A. C. Seydim, Development of Chitosan and Polycaprolactone based active bilayer films enhanced with nanocellulose and grape seed extract, Carbohyd. Polym. 195 (2018) 180-188.

DOI: 10.1016/j.carbpol.2018.04.071

Google Scholar

[6] N. E. Miri, K. Abdelouahdi, A. Barakat, M. Zahouily, A. Fihri, A. Solhy, M. E. Achaby, Bio-nanocomposite films reinforced with cellulose nanocrystals: Rheology of film-forming solutions, transparency, water vapor barrier and tensile properties of films, Carbohyd. Polym. 129 (2015) 156-167.

DOI: 10.1016/j.carbpol.2015.04.051

Google Scholar

[7] K. H. A. Hamid, N. A. M. Z.Saupy, N. M. Zain, S. K. A. Mudalip, S. M. Shaarani, N. A. M. Azman, Development and characterization of semi-refined carrageenan (SRC) films from Eucheuma cottonii incorporated with glycerol and α-tocopherol for active food packaging application, in IOP Conference Series: Mater. Sci. Eng. 458 (2018).

DOI: 10.1088/1757-899x/458/1/012022

Google Scholar

[8] J. H. Li, J. Miao, J. L. Wu, S. F. Chen, Q. Q. Zhang, Preparation and characterization of active gelatin-based films incorporated with natural antioxidants, Food Hydrocolloids, 37 (2014) 166-173.

DOI: 10.1016/j.foodhyd.2013.10.015

Google Scholar

[9] N. F. R. Nazurah, Z. Hanani, Physicochemical characterization of kappa-carrageenan (Euchema cottoni) based films incorporated with various plant oils, Carbohyd. Polym. 157 (2017) 1479-1487.

DOI: 10.1016/j.carbpol.2016.11.026

Google Scholar

[10] K. Harini, C. C. Mohan, K. Ramya, S. Karthikeyan, M. Sukumar, Effect of Punica granatum peel extracts on antimicrobial properties in Walnut shell cellulose reinforced Bio-thermoplastic starch films from cashew nut shells, Carbohyd. Polym. 184 (2018) 231-242.

DOI: 10.1016/j.carbpol.2017.12.072

Google Scholar

[11] Y. Zhao, R. R. Huerta, M. D. A. Saldaña, Use of subcritical water technology to develop cassava starch/chitosan/gallic acid bioactive films reinforced with cellulose nanofibers from canola straw, J. Supercritic. Fluids, 148 (2019) 55-65.

DOI: 10.1016/j.supflu.2019.02.022

Google Scholar

[12] Y. Xu, X. Ren, M. A. Hanna, Chitosan/clay nanocomposite film preparation and characterization, J. Appl. Polym. Sci. 99 (2006) 1684-1691.

DOI: 10.1002/app.22664

Google Scholar

[13] M. N. Angles, A. Dufresne, Plasticized starch/tunicin whiskers nanocomposite materials. 2. Mechanical behavior, Macromolecules, 34 (2001) 2921-2931.

DOI: 10.1021/ma001555h

Google Scholar

[14] B. Cuq, N. Gontard, J. L. Cuq, S. Guilbert, Functional properties of myofibrillar protein‐based biopackaging as affected by film thickness, J. food sci. 61 (1996) 580-584.

DOI: 10.1111/j.1365-2621.1996.tb13163.x

Google Scholar

[15] Z. Yu, F. K. Alsammarraie, F. X. Nayigiziki, W. Wang, B. Vardhanabhuti, A. Mustapha, M. Lin, Effect and mechanism of cellulose nanofibrils on the active functions of biopolymer-based nanocomposite films, Food Res. Int. 99 (2017) 166-172.

DOI: 10.1016/j.foodres.2017.05.009

Google Scholar

[16] R. Priyadarshi, Sauraj, B. Kumar, Y. S. Negi, Chitosan film incorporated with citric acid and glycerol as an active packaging material for extension of green chilli shelf life, Carbohyd. Polym. 195 (2018) 329-338.

DOI: 10.1016/j.carbpol.2018.04.089

Google Scholar

[17] H. W. Kwak, H. Lee, M. E. Lee, H. J. Jin, Facile and green fabrication of silk sericin films reinforced with bamboo-derived cellulose nanofibrils, J. Cleaner Product. 200 (2018) 1034-1042.

DOI: 10.1016/j.jclepro.2018.07.289

Google Scholar