Anisotropy in Third-Order Nonlinear Optical Susceptibility of the Stretch-Oriented Chrysophenine-Doped Poly(vinyl alcohol) Films

Zhao Hui Jin; Hua Jing Gao

doi:10.4028/www.scientific.net/AMR.634-638.2432

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HomeAdvanced Materials ResearchAdvanced Materials Research Vols. 634-638Anisotropy in Third-Order Nonlinear Optical...

Anisotropy in Third-Order Nonlinear Optical Susceptibility of the Stretch-Oriented Chrysophenine-Doped Poly(vinyl alcohol) Films

Abstract:

Stretch-oriented chrysophenine-doped poly(vinyl alcohol) (PVA) films were prepared at temperatures above the glass transition temperature of PVA. The optical absorption spectra of the stretch-oriented films exhibited a very high anisotropy (anisotropy ratio = 13). The third-order nonlinear optical properties of chrysophenine in stretch-oriented PVA films were measured by the resonant femtosecond degenerate four-wave mixing (DFWM) technique. The anisotropy ratio of the DFWM signal intensity was greater than 1000. The value of third-order nonlinear optical susceptibility of a uniaxially stretch-oriented chrysophenine-doped PVA film was 6.9×10^-13 esu.

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Advanced Materials Research (Volumes 634-638)

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2432-2435

DOI:

https://doi.org/10.4028/www.scientific.net/AMR.634-638.2432

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Online since:

January 2013

Authors:

Zhao Hui Jin, Hua Jing Gao

Keywords:

Chrysophenine, Degenerate Four-Wave Mixing, Resonant Conditions, Stretch-Oriented Film, Third-Order Nonlinear Optical Susceptibility

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