Field Methane Oxidation Efficiency at Municipal Solid Waste Landfills Located in the North of China

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Municipal solid waste (MSW) landfills are one of main sources of anthropogenic methane emissions in China, and methane has been predicted to be the most significant greenhouse gas after 2030. In landfills, oxidation can take place naturally with methane migrating through the landfill cover. The value of fraction of methane oxidation recommended by the US EPA is 10%, which, however, is being challenged with more and more field measurement data from the Europe and the US. The characteristic of MSW in China is extremely different from that in the US, probably resulting in distinct differences in both methane generation and oxidation. The objective of this study was to determine the fraction of methane oxidized at MSW landfills in China and its spatial and temporal variations. Stable isotope technique was applied to determine the fraction of methane oxidized. The results showed that the fraction of methane oxidized where MSW was covered by soil ranged from 6.3% to 100% in Northeast China and 31% to 100% in North China. Methane oxidation could hardly occur in the operating surface. Besides, soil cover always had a high methane oxidation efficiency in summer. The fractional oxidation of methane in summer was more than 2 times than that in winter. All over the year, with the sampling depth decreasing, the fraction of methane oxidation of soil cover increased.

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812-820

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January 2014

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[1] P. Forster, V. Ramaswamy, P. Artaxo, T. Berntsen, R. Betts, D.W. Fahey, J. Haywood, J. Lean, D.C. Lowe and G. Myhre, Changes in atmospheric constituents and in radiative forcing, Climate change 20 (2007).

Google Scholar

[2] IPCC (2007).

Google Scholar

[3] C. Scheutz, P. Kjeldsen, J.E. Bogner, A. De Visscher, J. Gebert, H.A. Hilger, M. Huber-Humer and K. Spokas, Microbial methane oxidation processes and technologies for mitigation of landfill gas emissions, Waste Manage Res. 27 (2009) 409-455.

DOI: 10.1177/0734242x09339325

Google Scholar

[4] EPA(Environmental Protection Agency) (2012) Inventory Of U.S. Greenhouse Gas Emissions And Sinks: 1990 – 2010, EPA 430-R-12-001, USA. Available from: http: /www. epa. gov /climatechange/Downloads/ghgemissions/US-GHG-Inventory-2012-Main-Text. pdf.

Google Scholar

[5] EEA (European Environment Agency) (2008) Annual European Community Greenhouse Gas Inventory 1990–2006 and Inventory Report 2008. Submission to the UNFCCC Secretariat. EEA Technical report, no. 6. 2008. ISSN 1725-2237.

Google Scholar

[6] J.E. Bogner, K.A. Spokas and E.A. Burton, Kinetics of methane oxidation in a landfill cover soil: temporal variations, a whole-landfill oxidation experiment, and modeling of net CH4 emissions, Environ Sci Technol. 31 (1997) 2504-2514.

DOI: 10.1021/es960909a

Google Scholar

[7] C. Scheutz, H. Mosbæk and P. Kjeldsen, Attenuation of methane and volatile organic compounds in landfill soil covers, J Environ Qual. 33 (2004) 61-71.

DOI: 10.2134/jeq2004.6100

Google Scholar

[8] V.B. Stein and J. Hettiaratchi, Methane oxidation in three Alberta soils: influence of soil parameters and methane flux rates, Environ Technol. 22 (2001) 101-111.

DOI: 10.1080/09593332208618315

Google Scholar

[9] J.M. Einola, R.H. Kettunen and J.A. Rintala, Responses of methane oxidation to temperature and water content in cover soil of a boreal landfill, Soil Biology and Biochemistry. 39 (2007) 1156-1164.

DOI: 10.1016/j.soilbio.2006.12.022

Google Scholar

[10] J. Chanton and K. Liptay, Seasonal variation in methane oxidation in a landfill cover soil as determined by an in situ stable isotope technique, Global Biogeochem Cy. 14 (2000) 51-60.

DOI: 10.1029/1999gb900087

Google Scholar

[11] T. Abichou, D. Powelson, J. Chanton, S. Escoriaza and J. Stern, Characterization of methane flux and oxidation at a solid waste landfill, Journal of Environmental Engineering. 132 (2006) 220-228.

DOI: 10.1061/(asce)0733-9372(2006)132:2(220)

Google Scholar

[12] T. Abichou, J. Clark and J. Chanton, Reporting central tendencies of chamber measured surface emission and oxidation, Waste Manage. 31 (2011) 1002-1008.

DOI: 10.1016/j.wasman.2010.09.014

Google Scholar

[13] J. Chanton, T. Abichou, C. Langford, G. Hater, R. Green, D. Goldsmith and N. Swan, Landfill Methane Oxidation Across Climate Types in the U.S., Environ Sci Technol. 45 (2010) 313-319.

DOI: 10.1021/es101915r

Google Scholar

[14] T. Abichou, L. Yuan and J. Chanton, Estimating methane emission and oxidation from earthen landfill covers. In: GeoCongress 2008: Geotechnics of Waste Management and Remediation, March 9, 2008 - March 12, 2008 (American Society of Civil Engineers, New Orleans, LA, United states, 2008), pp.80-87.

DOI: 10.1061/40970(309)10

Google Scholar

[15] T. Abichou, J. Chanton, D. Powelson, J. Fleiger, S. Escoriaza, Y. Lei and J. Stern, Methane flux and oxidation at two types of intermediate landfill covers, Waste Manage. 26 (2006) 1305-1312.

DOI: 10.1016/j.wasman.2005.11.016

Google Scholar

[16] J.P. Chanton, D.K. Powelson, T. Abichou and G. Hater, Improved field methods to quantify methane oxidation in landfill cover materials using stable carbon isotopes, Environ Sci Technol. 42 (2007) 665-670.

DOI: 10.1021/es0710757

Google Scholar

[17] J. Chanton, D. Powelson and R. Green, Methane Oxidation in Landfill Covers Soils. (ASCE, 2009), pp.2896-2905.

Google Scholar

[18] J.P. Chanton, D.K. Powelson, T. Abichou, D. Fields and R. Green, Effect of temperature and oxidation rate on carbon-isotope fractionation during methane oxidation by landfill cover materials, Environ Sci Technol. 42 (2008) 7818-7823.

DOI: 10.1021/es801221y

Google Scholar

[19] M.A. Barlaz, R.B. Green, J.P. Chanton, C.D. Goldsmith and G.R. Hater, Evaluation of a Biologically Active Cover for Mitigation of Landfill Gas Emissions, Environ Sci Technol. 38 (2004) 4891-4899.

DOI: 10.1021/es049605b

Google Scholar

[20] W. Chiemchaisri, C. Chiemchaisri and J. Boonchaiyuttasak, Utilization of stabilized wastes for reducing methane emission from municipal solid waste disposal, Bioresource Technol. 141 (2013) 199-204.

DOI: 10.1016/j.biortech.2013.03.035

Google Scholar

[21] G. Börjesson, I. Sundh and B. Svensson, Microbial oxidation of CH4 at different temperatures in landfill cover soils, Fems Microbiol Ecol. 48 (2004) 305-312.

DOI: 10.1016/j.femsec.2004.02.006

Google Scholar

[22] V.B. Stein and J. Hettiaratchi, Methane oxidation in three Alberta soils: influence of soil parameters and methane flux rates, Environ Technol. 22 (2001) 101-111.

DOI: 10.1080/09593332208618315

Google Scholar

[23] J. Park, S. Moon, Y.M. Ahn, J.Y. Kim and K. Nam, Determination of environmental factors influencing methane oxidation in a sandy landfill cover soil, Environ Technol. 26 (2005) 93-102.

DOI: 10.1080/09593332608618586

Google Scholar