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Promoting Effect of CeO2 Addition on Activity and Catalytic Stability in Steam Reforming of Methane over Ni/Al2O3

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Abstract:

Hydrogen production by steam reforming of methane was studied over Ni catalysts supported on CeO2, Al2O3 and CeO2-Al2O3. These catalysts were prepared using the impregnation method and characterized by XRD. The effect of CeO2 promoter on the catalytic performance of Ni/Al2O3 catalyst for methane steam reforming reaction was investigated. In fact, CeO2 had a positive effect on the catalytic activity in this reaction. Experimental results demonstrated that Ni/CeO2-Al2O3 catalyst showed excellent catalytic activity and high reaction performance. In addition, the effects of reaction temperature and metal content on the conversion of CH4 and H2/CO ratio were also investigated. Results indicated that CH4 conversion increased significantly with the increase of the reaction temperature and metal content.

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Periodical:

Advanced Materials Research (Volume 324)

Pages:

153-156

DOI:

https://doi.org/10.4028/www.scientific.net/AMR.324.153

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Online since:

August 2011

Authors:

Abdelmajid Rakib, Cédric Gennequin, Thierry Dhainaut, Sylvain Ringot, Antoine Aboukaïs, Edmond Abi-Aad

Keywords:

CeO2-Al2O3, Hydrogen Production, Nickel Catalysts, Steam Reforming of Methane

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© 2011 Trans Tech Publications Ltd. All Rights Reserved

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