Resonant Third-Order Optical Nonlinearities of the Stretch-Oriented Cyanine-Dye-Doped Poly(vinyl Alcohol) Films

Zhao Hui Jin; Hua Jing Gao; Yong Wu Han

doi:10.4028/www.scientific.net/AMR.476-478.1237

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HomeAdvanced Materials ResearchAdvanced Materials Research Vols. 476-478Resonant Third-Order Optical Nonlinearities of the...

Resonant Third-Order Optical Nonlinearities of the Stretch-Oriented Cyanine-Dye-Doped Poly(vinyl Alcohol) Films

Abstract:

Stretch-oriented cyanine-dye-doped poly(vinyl alcohol) (PVA) films were prepared at temperatures above the glass transition temperature of PVA. The optical absorption spectra of the stretch-oriented films exhibited an anisotropy. The third-order nonlinear optical susceptibilities of the stretch-oriented films were measured parallel and perpendicular to the stretching direction by the resonant femtosecond degenerate four-wave mixing (DFWM) technique, and a high anisotropic X⁽³⁾ was observed for the uniaxially stretch-oriented cyanine-dye-doped PVA films.

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Periodical:

Advanced Materials Research (Volumes 476-478)

Pages:

1237-1240

DOI:

https://doi.org/10.4028/www.scientific.net/AMR.476-478.1237

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Online since:

February 2012

Authors:

Zhao Hui Jin, Hua Jing Gao, Yong Wu Han

Keywords:

Degenerate Four-Wave Mixing (DFWM), Optical Absorption Anisotropy, Stretch-Oriented Film, Third-Order Nonlinear Optical Susceptibility

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