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Effects of Carriers on Amination of Ethanol to Acetonitrile over Catalysts Loaded with Cu

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Abstract:

In this study, we first purposefully synthesized SAPO-11 and Na-ZSM-23 molecular sieves. The catalysts loaded with Cu were prepared by using seven typical carriers, including Montmorillonite-K10, USY, SAPO-11, Na-ZSM-23, γ-Al2O3, ZnO and MgO, and the performance of the catalysts was tested for amination of ethanol. The results demonstrate that the acid-base property of the carriers is closely related with the results of amination of ethanol over the catalysts. Among all these catalysts, 15%Cu/Na-ZSM-23 shows the highest yield of acetonitrile.

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Periodical:

Advanced Materials Research (Volumes 750-752)

Pages:

1700-1703

DOI:

https://doi.org/10.4028/www.scientific.net/AMR.750-752.1700

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Online since:

August 2013

Authors:

Jun Deng, Hong Sheng Zhang, Yun Feng Hu, Ying Liu, Dan Dan Wang

Keywords:

Acetonitrile, Carrier, Ethanol, Na-ZSM-23

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© 2013 Trans Tech Publications Ltd. All Rights Reserved

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