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Highly Active Fischer-Tropsch Synthesis Fe-BDC MOF-Derived Catalyst Prepared by Modified Solvothermal Method

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Abstract:

Fe-MIL-88B was prepared by a method that utilizes ferric nitrate and terephthalic acid (TPA or H2BDC) as precursors. The catalyst was characterized by TEM, SEM, FTIR, XRD, BET, and TGA. The pyrolyzed MOF (Fe-MIL-88B/C) was then tested for FTS at 300 psi, 300/340°C and H2/CO=1 after reduction under flow of hydrogen at 400°C for 4 hours. GC product results show promising FTS performance and stability compared to previously reported Fe-MOF derived catalysts with CO conversion of 96.90% at 340°C for 40 hours and 97.45% at 300°C for 26 hours.

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Periodical:

Key Engineering Materials (Volume 891)

Pages:

56-61

DOI:

https://doi.org/10.4028/www.scientific.net/KEM.891.56

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Online since:

July 2021

Authors:

Ahmed Elsayed Rashed*, Kamal Essam, Marwa F. El Kady, Matsushita Yoshihisa, Ahmed Abd El-Moneim, AL-Hassan Mohammed Nasser

Keywords:

Catalysis, Fischer-Tropsch Synthesis, Iron-Based Catalyst, Metal-Organic Frameworks

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© 2021 Trans Tech Publications Ltd. All Rights Reserved

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