In Situ and Real-Time Analysis of TEM Forces Induced by a Permanent Magnetic Field during Solidification of Al-4wt%Cu

Article Preview

Abstract:

It is well known that the application of a magnetic field during the growth process can have pronounced effects on cast material structures and their properties, so that magnetic fields have been widely applied since the 1950s. In the case of a permanent magnetic field, some recent results revealed a dual effect on the liquid metal flow. 1: the magnetic field has a selective damping action on the flow at the scale of the crucible, due to the Lorentz force; 2: the interaction of thermo-electro-magnetic (TEM) currents in the close vicinity of the solid-liquid interface with the applied magnetic field leads to the generation of electromagnetic forces, which act both on the liquid and on the solid at the scale of the microstructure. We present an experimental investigation of the TEM forces induced by a permanent magnetic field during columnar and equiaxed solidification of Al-4wt%Cu. In situ visualization was carried out by means of synchrotron X-ray radiography, which is a method of choice for studying dynamic phenomena. It was shown that the TEM forces were at the origin of a motion of dendritic particles, perpendicular to the direction of gravity. A heuristic analysis allowed us to estimate the fluid velocities and the velocities of the solid particles, and a good agreement was achieved with the experimental data. Similar observations were also made during equiaxed growth in a temperature gradient. The in situ observation of the grain trajectories for various values of the temperature gradient demonstrated that gravity and TEM forces were the driving forces which controlled the grain motion.

You might also be interested in these eBooks

Info:

* - Corresponding Author

[1] J.A. Spittle, Columnar to equiaxed grain transition in as solidified alloys, International Materials Reviews, 51 (2006) 247-269.

DOI: 10.1179/174328006x102493

Google Scholar

[2] J.S. Langer, Dynamics of dendritic pattern formation, Materials Science and Engineering, 65 (1984) 37-44.

Google Scholar

[3] H. Nguyen-Thi, et al., Investigation of gravity effects on solidification of binary alloys with in situ X-ray radiography on earth and in microgravity environment, Journal of Physics: Conference Series, 327 (2011) 012012.

DOI: 10.1088/1742-6596/327/1/012012

Google Scholar

[4] A. Bogno, et al., Analysis by synchrotron X-ray radiography of convection effects on the dynamic evolution of the solid-liquid interface and on solute distribution during the initial transient of solidification, Acta Materialia, 59 (2011).

DOI: 10.1016/j.actamat.2011.03.059

Google Scholar

[5] G. Reinhart, et al., Investigation of Columnar-Equiaxed Transition and Equiaxed growth of Aluminium Based Alloys by X-Ray Radiography, Materials Science and Engineering A, 413-414 (2005) 384-388.

DOI: 10.1016/j.msea.2005.08.197

Google Scholar

[6] G. Reinhart, et al., In-Situ and real-time analysis of the formation of strains and microstructure defects during solidification of Al-3. 5 wt pct Ni alloys, Metallurgical and Materials Transactions a-Physical Metallurgy and Materials Science, 39A (2008).

DOI: 10.1007/s11661-007-9449-2

Google Scholar

[7] B. Drevet, et al., Solidification of Aluminum-Lithium Alloys near the Cell/Dendrite Transition - Influence of Solutal Convection, J. Crystal Growth, 218 (2000) 419-433.

DOI: 10.1016/s0022-0248(00)00567-4

Google Scholar

[8] H. Nguyen Thi, et al., Directional Solidification of Al-1. 5wt% Ni alloys under diffusion transport in space and fluid flow localisation on Earth, J. of Crystal Growth, 281 (2005) 654-668.

DOI: 10.1016/j.jcrysgro.2005.04.061

Google Scholar

[9] W. Bingbo, Unidirectional dendritic solidification under longitudinal resonant vibration, Acta metall. mater., 40 (1992) 2739-2751.

DOI: 10.1016/0956-7151(92)90344-e

Google Scholar

[10] R. Caram, et al., Directional solidifiation of Pb-Sn eutectic with vibration, J. Cryst. Growth, 114 (1991) 249-254.

DOI: 10.1016/0022-0248(91)90698-5

Google Scholar

[11] D.T.J. Hurle, R.W. Series, Use of a magnetic field in melt growth, North Holland, Amsterdam ed., (1994).

Google Scholar

[12] P. Rudolph, Travelling magnetic fields applied to bulk crystal growth from the melt: The step from basic research to industrial scale, J. Cryst. Growth, 310 (2008) 1298-1306.

DOI: 10.1016/j.jcrysgro.2007.11.036

Google Scholar

[13] P.A. Davidson, Magnetohydrodynamics in materials processing, Annual Review of Fluid Mechanics, 31 (1999) 273-300.

Google Scholar

[14] R. Moreau, Magnetohydrodynamics, Kluwer Publications, Dordrecht, The Netherlands, (1990).

Google Scholar

[15] J.A. Shercliff, Thermoelectric Magnetohydrodynamics, J. Fluid Mech., 91 (1979) 231-251.

DOI: 10.1017/s0022112079000136

Google Scholar

[16] P. Lehmann, et al., Modification of interdendritic convection in directional solidification by a uniform magnetic field, Acta Materialia, 46 (1998) 4067-4079.

DOI: 10.1016/s1359-6454(98)00064-0

Google Scholar

[17] H. Nguyen-Thi, et al., On the interest of synchrotron X-ray imaging for the study of solidification in metallic alloys, Comptes Rendus Physique, 13 (2012) 237-245.

DOI: 10.1016/j.crhy.2011.11.010

Google Scholar

[18] H. Nguyen Thi, et al., Preliminary in situ and real-time study of directional solidification of metallic alloys by X-ray imaging techniques, J. Phys. D: Appl. Phys., 36 (2003) A83-A86.

DOI: 10.1088/0022-3727/36/10a/317

Google Scholar

[19] J. Wang, et al., Thermoelectric magnetic force acting on the solid during directional solidification under a static magnetic field, Appl. Phys. Lett., 101 (2012).

Google Scholar

[20] H. Nguyen Thi, et al., Tailoring of Dendritic Microstructure in Solidification Processing By Crucible Vibration, J. of Crystal Growth, 275 (2005) 1579-1584.

DOI: 10.1016/j.jcrysgro.2004.11.223

Google Scholar

[21] S. Ganesan, D.R. Poirier, Densities of Aluminum-Rich Aluminum-Copper Alloys during Solidification, Metallurgical Transaction A, 18A (1987) 721-723.

DOI: 10.1007/bf02649490

Google Scholar