Investigation of In-Flight Annihilation of Positrons Using Coincidence Doppler Broadening Spectroscopy

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Doppler Broadening Spectroscopy (DBS) of the positron electron annihilation line allows the detection and analysis of defects in materials. DBS uses the fact that during the annihilation momentum has to be conserved and is therefore transferred from the annihilating positron-electron pair to the annihilation gamma quanta. As a sufficient approximation the positron is assumed to be thermalized in the solid when it annihilates with an electron. In that case, the dominant fraction of the transferred momentum originates from the electrons. However, when implanting high-energy positrons a small fraction of positrons (typicylly less than 1%) will annihilate with electrons before thermalizing. This process of in-flight annihilation can be differentiated from annihilation of thermalized positrons by Coincidence DBS (CDBS). We used the CDB Spectrometer at the NEutron induced POsitron source MUniCh (NEPOMUC) in order get a deeper understanding of in-flight annihilation in several materials of different densities and core annihilation probabilities. We utilized a 22Na source as positron emitter which not only provides insight into the thermalization process of positrons, but also extends the capabilities of the CDB spectrometer.

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Solid State Phenomena (Volume 374)

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3-12

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July 2025

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© 2025 Trans Tech Publications Ltd. All Rights Reserved

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[1] K.G. Lynn, et al. Positron-annihilation momentum profiles in aluminum: core contribution and the independent-particle model. Physical Review Letters 38.5 (1977): 241.

DOI: 10.1103/physrevlett.38.241

Google Scholar

[2] R. Krause-Rehberg and H.S. Leipner: Positron annihilation in semiconductors: defect studies (1999).

DOI: 10.1007/978-3-662-03893-2_8

Google Scholar

[3] W. Brandt and N. Arista: Thermalization and diffusion of positrons in solids Phys. Rev. B, Vol 26 (1982), p.4229.

DOI: 10.1103/physrevb.26.4229

Google Scholar

[4] H.W. Kendall, and M. Deutsch. Annihilation of positrons in flight. Physical Review 101.1 (1956): 20.

Google Scholar

[5] Č. Jakub, et al. Low background digital coincidence spectrometer–a tool for investigation of positron annihilation in flight. Defect and Diffusion Forum. Vol. 331 (2012), Trans Tech Publications Ltd.

DOI: 10.4028/www.scientific.net/ddf.331.53

Google Scholar

[6] Č. Jakub, et al. Investigation of positron annihilation-in-flight using a digital coincidence Doppler broadening spectrometer. New Journal of Physics 14.3 (2012): 035005.

DOI: 10.1088/1367-2630/14/3/035005

Google Scholar

[7] M.J. Berger and S.M. Seltzer: Tables of energy losses and ranges of electrons and positrons No. NASA-SP-3012 (1964).

Google Scholar

[8] A. Perkins and JP. Carbotte: Effect of the Positron-Phonon Interaction on Positron Motion Phys. Rev. B, Vol. 1 (1970), p.101.

DOI: 10.1103/physrevb.1.101

Google Scholar

[9] K.O. Jensen and A. Weiss. Theoretical study of the application of positron-induced Augerelectron spectroscopy. Physical Review B 41.7 (1990): 3928.

Google Scholar

[10] P. Pikart and C. Hugenschmidt. Determination of electron binding energies in two-dimensional Coincident Doppler Broadening spectra. Journal of Physics: Conference Series. Vol. 443. No. 1. IOP Publishing, (2013).

DOI: 10.1088/1742-6596/443/1/012089

Google Scholar

[11] C. Hugenschmidt, et al.: The NEPOMUC upgrade and advanced positron beam experiments. New Journal of Physics, 14.5 (2012): 055027.

DOI: 10.1088/1367-2630/14/5/055027

Google Scholar

[12] T. Gigl, et al. Defect imaging and detection of precipitates using a new scanning positron microbeam. New Journal of Physics 19.12 (2017): 123007.

DOI: 10.1088/1367-2630/aa915b

Google Scholar